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• W2012191034 abstract "The electron density in each of the outermost molecular orbitals of NH2CH3, NH (CH3)2, N(CH3)3 and NF3, as probed by electron momentum spectroscopy, is found to exhibit a very much higher degree of s character than the corresponding orbital in NH3. Increasing methyl substitution in NH3 results in increasing amounts of s character in the experimental momentum profiles. This trend is qualitatively predicted by MO calculations which indicate appreciable delocalization of electron density away from the nitrogen in the methyl amines and NF3. The relevance of the present results to current understanding of the methyl inductive effect is discussed." @default.
• W2012191034 created "2016-06-24" @default.
• W2012191034 creator A5027307728 @default.
• W2012191034 creator A5072460099 @default.
• W2012191034 date "1988-06-01" @default.
• W2012191034 modified "2023-09-27" @default.
• W2012191034 title "Studies of the electron density in the outermost orbitals of NH2CH3, NH(CH3)2, N(CH3)3 and NF3 by electron momentum spectroscopy: Evidence for charge delocalization" @default.
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• W2012191034 doi "https://doi.org/10.1016/0301-0104(88)87031-9" @default.
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