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- W2012195059 abstract "Abstract A novel tripyridylporphyrin monomer, 5-[4-[2-(acryloyloxy)ethoxy]phenyl]-10,15,20-tris(4-pyridyl)porphyrin (TrPyP), and its zinc (II) complex (ZnTrPyP) were synthesized. It was copolymerized with acrylamide to prepare water-soluble polymer P(ZnTrPyP-AM). The aggregation behavior of P(ZnTrPyP-AM) in aqueous solution was investigated by UV–visible absorption spectra. The red shift of Q band and the significantly enhanced relative intensity ( ɛ α / ɛ β ) indicated that the ZnTrPyP was axially coordinated. Meanwhile, Soret band of porphyrin split into two bands, suggesting exciton coupling of aggregates. The porphyrin pendants of P(ZnTrPyP-AM) were supposed to form a slipped cofacial dimer and the macromolecular matrix helped to create the well-defined porphyrin aggregates. This finding was helpful for the assembly of artificial light-harvesting systems in aquatic environment to mimic the dimeric structure in natural LHC." @default.
- W2012195059 created "2016-06-24" @default.
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- W2012195059 date "2011-04-01" @default.
- W2012195059 modified "2023-10-17" @default.
- W2012195059 title "The formation of a slipped cofacial dimer of zinc (II) tripyridylporphyrin in water-soluble polymer" @default.
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- W2012195059 doi "https://doi.org/10.1016/j.jphotochem.2011.03.020" @default.
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