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- W2012203265 abstract "A Hygroscopicity Tandem Differential Mobility Analyzer (H-TDMA) system has been used to measure hygroscopic growth curves and deliquescence relative humidities (DRH) of laboratory generated (NH4)2SO4, NaCl, and NaNO3 particles at temperatures T= 20 degrees C and -10 degrees C. Good agreement (better than 3.5%) between measured growth curves and Köhler theory was found using empirical temperature and concentration dependent values for water activity, solution density, and surface tension. The measured growth curves only experience a small temperature dependence in the observed temperature range. Therefore, to a first approximation, it is possible to neglect the temperature dependence of the water activity for theoretical calculations in the temperature range -10 degrees C < T < 25 degrees C. The small differences between experiment and theory, which were predominantly observed for NaCl particles, are probably caused by a small amount of water adsorbed on the dry crystals. It was also observed that these particles experience a significant restructuring at relative humidity RH < DRH, which was also taken into account for a comparison with theoretical curves. If salt particles are used for instrument calibration, precautions regarding the dry particle diameter have to be taken." @default.
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- W2012203265 date "2001-11-21" @default.
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- W2012203265 title "Hygroscopicity of Aerosol Particles at Low Temperatures. 2. Theoretical and Experimental Hygroscopic Properties of Laboratory Generated Aerosols" @default.
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- W2012203265 doi "https://doi.org/10.1021/es010055g" @default.
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