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- W2012211558 abstract "Mononuclear nonheme iron(IV)-oxo complexes with two different topologies, cis-α-[FeIV(O)(BQCN)]2+ and cis-β-[FeIV(O)(BQCN)]2+, were synthesized and characterized with various spectroscopic methods. The effect of ligand topology on the reactivities of nonheme iron(IV)-oxo complexes was investigated in C–H bond activation and oxygen atom-transfer reactions; cis-α-[FeIV(O)(BQCN)]2+ was more reactive than cis-β-[FeIV(O)(BQCN)]2+ in the oxidation reactions. The reactivity difference between the cis-α and cis-β isomers of [FeIV(O)(BQCN)]2+ was rationalized with the FeIV/III redox potentials of the iron(IV)-oxo complexes: the FeIV/III redox potential of the cis-α isomer was 0.11 V higher than that of the cis-β isomer." @default.
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- W2012211558 date "2011-07-15" @default.
- W2012211558 modified "2023-10-16" @default.
- W2012211558 title "Ligand Topology Effect on the Reactivity of a Mononuclear Nonheme Iron(IV)-Oxo Complex in Oxygenation Reactions" @default.
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- W2012211558 doi "https://doi.org/10.1021/ja204008u" @default.
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