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- W2012259640 abstract "Abstract We report on a novel spin–lattice phase transition in an ionic mixed-stack charge-transfer (CT) compound of (BEDO-TTF)(Cl 2 TCNQ). We found that the rotational modes for rigid-body displacements of molecules afforded an appreciable quantitative variation in the exchange interactions along the mixed stacks, which resulted in the symmetry - invariant first-order magneto-lattice phase transition at around 110 K. It was found in the electron paramagnetic resonance (EPR) spectra that the low-temperature strongly interacting spin phase was followed by a magnetic order at 16 K. We discuss the origin of the transition at 110 K in terms of the competition of free energy between the respective spin states. We also present neutral–ionic (NI) phase transition in the isomorphous compound of (BEDT-TTF)(ClMeTCNQ) under pressure." @default.
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- W2012259640 date "2003-03-01" @default.
- W2012259640 modified "2023-10-18" @default.
- W2012259640 title "Novel magneto-lattice transition in the mixed-stack charge-transfer complexes with inter-columnar networks" @default.
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- W2012259640 doi "https://doi.org/10.1016/s0379-6779(02)00364-8" @default.
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