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• W2012306680 abstract "For multidimensional activated rate processes controlled by diffusive crossing of a saddle point region, we show that a one-dimensional reaction coordinate can be constructed even when the diffusion anisotropy is arbitrary. The rate constant, found using the potential of mean force along this coordinate, is identical to that predicted by the multidimensional Kramers-Langer theory. This reaction coordinate minimizes the one-dimensional rate constant obtained using a trial reaction coordinate and is orthogonal to the stochastic separatrix, the transition state that separates reactants from products." @default.
• W2012306680 created "2016-06-24" @default.
• W2012306680 creator A5039584452 @default.
• W2012306680 creator A5053509000 @default.
• W2012306680 date "2004-12-13" @default.
• W2012306680 modified "2023-09-26" @default.
• W2012306680 title "One-dimensional reaction coordinates for diffusive activated rate processes in many dimensions" @default.
• W2012306680 cites W1966036962 @default.
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• W2012306680 doi "https://doi.org/10.1063/1.1818091" @default.
• W2012306680 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/15638670" @default.
• W2012306680 hasPublicationYear "2004" @default.
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