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- W2012322128 abstract "Gas-phase room-temperature methane activation by various clusters draws increasing attention. In this Letter, we produce a series of bimetallic oxide clusters which contain both main-group metal aluminum atoms and transition-metal vanadium atoms. We provide solid experimental and theoretical evidence that bimetallic AlVO4+ cluster can draw a hydrogen atom from methane to produce CH3 at room temperature. The Al3VO7+ cluster which can be considered as a system formed from Al2O3 + AlVO4+ does not break C–H bonds of methane. The results enrich the chemistry of gas phase methane activation and provide possible molecular level mechanism to couple with heterogeneous catalysis." @default.
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- W2012322128 date "2010-04-01" @default.
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- W2012322128 title "Room-temperature methane activation by a bimetallic oxide cluster <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML altimg=si1.gif display=inline overflow=scroll><mml:mrow><mml:msubsup><mml:mrow><mml:mtext>AlVO</mml:mtext></mml:mrow><mml:mrow><mml:mn>4</mml:mn></mml:mrow><mml:mrow><mml:mo>+</mml:mo></mml:mrow></mml:msubsup></mml:mrow></mml:math>" @default.
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- W2012322128 doi "https://doi.org/10.1016/j.cplett.2010.02.040" @default.
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