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• W2012324053 abstract "Adsorption of CO on Ni(111) surfaces was studied by means of LEED, UPS and thermal desorption spectroscopy. On an initially clean surface adsorbed CO forms a √3 × √3R30° structure at θ = 0.33 whose unit cell is continuously compressed with increasing coverage leading to a c4 × 2-structure at θ = 0.5. Beyond this coverage a more weakly bound phase characterized by a √72 × √72R19° LEED pattern is formed which is interpreted with a hexagonal close-packed arrangement (θ = 0.57) where all CO molecules are either in “bridge” or in single-site positions with a mutual distance of 3.3 Å. If CO is adsorbed on a surface precovered by oxygen (exhibiting an O 2 × 2 structure) a partially disordered coadsorbate 2 × 2 structure with θo = θco = 0.25 is formed where the CO adsorption energy is lowered by about 4 kcal/mole due to repulsive interactions. In this case the photoemission spectrum exhibits not a simple superposition of the features arising from the single-component adsorbates (i.e. maxima at 5.5 eV below the Fermi level with Oad, and at 7.8 (5σ + 1π) and 10.6 eV (4σ) with COad, respectively), but the peak derived from the CO 4σ level is shifted by about 0.3 eV towards higher ionization energies." @default.
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• W2012324053 date "1976-07-01" @default.
• W2012324053 modified "2023-10-03" @default.
• W2012324053 title "Adsorption of CO on clean and oxygen covered Ni(111) surfaces" @default.
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• W2012324053 doi "https://doi.org/10.1016/0039-6028(76)90341-1" @default.
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