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• W2012387611 abstract "We propose a two-step protocol for inverting ultrafast spectroscopy experiments on a molecular aggregate to extract the time-evolution of the excited state density matrix. The first step is a deconvolution of the experimental signal to determine a pump-dependent response function. The second step inverts this response function to obtain the quantum state of the system, given a model for how the system evolves following the probe interaction. We demonstrate this inversion analytically and numerically for a dimer model system, and evaluate the feasibility of scaling it to larger molecular aggregates such as photosynthetic protein-pigment complexes. Our scheme provides a direct alternative to the approach of determining all Hamiltonian parameters and then simulating excited state dynamics." @default.
• W2012387611 created "2016-06-24" @default.
• W2012387611 creator A5019265176 @default.
• W2012387611 creator A5070161680 @default.
• W2012387611 date "2013-04-22" @default.
• W2012387611 modified "2023-10-16" @default.
• W2012387611 title "Inverting pump-probe spectroscopy for state tomography of excitonic systems" @default.
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• W2012387611 doi "https://doi.org/10.1063/1.4800800" @default.
• W2012387611 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/23635106" @default.
• W2012387611 hasPublicationYear "2013" @default.
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