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• W2012596626 endingPage "2228" @default.
• W2012596626 startingPage "2219" @default.
• W2012596626 abstract "Various cobalt complexes of 4,10-dipropyl-5,9-diazatrideca-4,9-diene-3,10-dione dioxime, (C2C3)(DOH)2pn, were prepared, and redox behavior of them was investigated by means of cyclic voltammetry; Co(II)/Co(I) redox potentials in the range of −0.69 through −0.7 V vs. Ag/AgCl. The monomethylated complex, which has a cobalt–carbon bond at one axial site of the nuclear cobalt, was disproportionated to the dimethylated complex, involving two cobalt–carbon bonds at both axial sites, and the CoI species by one-electron reduction. The dimethylated complex was inactive for electrochemical reduction, but transformed into the monomethylated complex via cleavage of a cobalt–carbon bond upon electrochemical oxidation. The electrolyses of 1-bromo-2,2-bis(ethoxycarbonyl)propane, 1-bromo-2-cyano-2-ethoxycarbonylpropane, and 2-acetyl-1-bromo-2-ethoxycarbonylpropane in the presence of [CoIII{(C2C3)(DO)(DOH)pn}Br2] in N,N-dimethylformamide did not proceed in a divided cell at −2.0 V vs. Ag/AgCl, since the corresponding dial..." @default.
• W2012596626 created "2016-06-24" @default.
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• W2012596626 date "1989-07-01" @default.
• W2012596626 modified "2023-10-18" @default.
• W2012596626 title "Redox Behavior of Simple Vitamin B₁₂Model Complexes and Electrochemical Catalysis of Carbon-Skeleton Rearrangements" @default.
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• W2012596626 doi "https://doi.org/10.1246/bcsj.62.2219" @default.
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