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- W2012805931 abstract "The temperature dependency of the oxygen quenching of the singlet excited states of both pyrene and 9,10-diphenylanthracene on nonporous silica gel has been studied by both laser-induced time-resolved and steady-state fluorescence spectroscopy. A Gaussian distribution of rate constants is presented to account for the heterogeneous kinetics. Oxygen adsorption isotherms on the silica gel surface above the gas/liquid critical temperature are determined; oxygen assimilation times of 23.2, 44.2, 99.5, and 238 ps have been calculated at {minus}47, {minus}64, {minus}80, and {minus}98{degree}C, respectively. A dynamic Langmuir-Hinshelwood model for the bimolecular quenching reaction is presented." @default.
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- W2012805931 date "1990-05-01" @default.
- W2012805931 modified "2023-09-25" @default.
- W2012805931 title "Gaussian approximation to the unique heterogeneous Langmuir-Hinshelwood type fluorescence quenching at the silica gel gas/solid interface: pyrene and 9,10-diphenylanthracene singlet quenching by oxygen" @default.
- W2012805931 doi "https://doi.org/10.1021/j100374a033" @default.
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