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- W2012862917 abstract "Oxygen Rydberg time-of-flight spectroscopy was used to study the vacuum ultraviolet photodissociation dynamics of N2O near 130 nm. The O(PJ3) products were tagged by excitation to high-n Rydberg levels and subsequently field ionized at a detector. In agreement with previous work, we find that O(PJ3) formation following excitation to the repulsive N2O D(Σ+1) state produces the first two electronically excited states of the N2 counterfragment, N2(AΣu+3) and N2(BΠg3). The O(PJ3) translational energy distribution reveals that the overall branching ratio between N2(AΣu+3) and N2(BΠg3) formation is approximately 1.0:1.0 for J=1 and 2, with slightly less N2(BΠg3) produced in coincidence with O(P03). The angular distributions were found to be independent of J and highly anisotropic, with β=1.5±0.2." @default.
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- W2012862917 date "2005-05-01" @default.
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- W2012862917 title "Photodissociation dynamics of N2O at 130 nm: The N2(AΣu+3,BΠg3)+O(PJ=2,1,3) channels" @default.
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- W2012862917 doi "https://doi.org/10.1063/1.1888578" @default.
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