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• W2012942500 abstract "The kinetics of the reaction of CCO radicals with NO and NO2 were studied using time-resolved infrared diode laser absorption spectroscopy. The rate constants were determined to be kCCO+NO = (5.36 ± 0.5) × 10-11 and kCCO+NO2 = (6.89 ± 0.5) × 10-11 cm3 molecule-1 s-1 at 298 K. These rate constants have virtually no temperature dependence over the range 298−573 K, with Arrhenius fits given by kCCO+NO = (1.66 ± 0.5) × 10-10 exp[(−337 ± 100)/T] and kCCO+NO2 = (8.51 ± 1.5) × 10-11 exp[(−63 ± 80)/T] (error bars represent one standard deviation). Product channel measurements were performed on the CCO + NO reaction. After consideration of secondary chemistry, we obtain the branching ratios φ(CN + CO2) = 0.13 ± 0.05 and φ(CO + NCO) = 0.87 ± 0.05 at 298 K. Ab initio quantum chemical calculations at the QCISD(T)/6-311G(2df,2pd) level of theory were used to examine probable reaction pathways." @default.
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• W2012942500 date "2003-12-04" @default.
• W2012942500 modified "2023-10-16" @default.
• W2012942500 title "Kinetics of the CCO + NO and CCO + NO₂ Reactions" @default.
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• W2012942500 doi "https://doi.org/10.1021/jp0304125" @default.
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