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- W2013000812 abstract "The new silanone complex 3 is accessible in 82% yield and is capable of undergoing addition of ammonia under mild conditions, yielding the sila-hemiaminal 4 and, at the same time, its unique tautomer 5, the first silanoic amide. The unexpected formation of 3 is due to the presence of the basic exocyclic methylene group in the C3N2 ligand backbone. Strikingly, the tautomers 4 and 5 are in equilibrium in solution and can be cocrystallized in benzene or THF solutions having a SiOH···O═Si hydrogen bond as confirmed by single-crystal X-ray diffraction analysis." @default.
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- W2013000812 date "2010-05-04" @default.
- W2013000812 modified "2023-10-14" @default.
- W2013000812 title "Activation of Ammonia by a Si═O Double Bond and Formation of a Unique Pair of Sila-Hemiaminal and Silanoic Amide Tautomers" @default.
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- W2013000812 doi "https://doi.org/10.1021/ja1031024" @default.
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