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- W2013055850 abstract "The weakly bound trimer between two argon atoms and a molecule of hydrogen bromide was identified from its rotational spectrum observed at conditions of supersonic expansion. The spectrum was measured with a cavity, Fourier transform microwave spectrometer and the rotational, quartic, and bromine hyperfine coupling constants were determined for the two most abundant isotopomers Ar402H79Br and Ar402H81Br. The various spectroscopic observables dependent on the harmonic force field were successfully reproduced using ab initio force field calculations. Experimental moments of inertia were then used, together with calculated vibration-rotation inertial contributions to derive the rz geometry. The resulting d(ArBr)=4.166 Å, d(ArAr)=3.840 Å, compare with rz distances d(ArBr)=4.155 Å for ArHBr, and d(ArAr)=3.836 Å for Ar2. Angular information derived from the measured nuclear hyperfine splitting constants and from the electric dipole moment was found to be in remarkable agreement. Comparisons of the available information on the interaction energy and geometries for the ArHX and the Ar2HX series of clusters have been made in order to assess the relationship between the experimental ground state based structural parameters and the desired equilibrium geometry." @default.
- W2013055850 created "2016-06-24" @default.
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- W2013055850 creator A5041861765 @default.
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- W2013055850 date "2002-10-22" @default.
- W2013055850 modified "2023-09-24" @default.
- W2013055850 title "The observation and characterization by rotational spectroscopy of the weakly bound trimer Ar2HBr" @default.
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- W2013055850 doi "https://doi.org/10.1063/1.1511182" @default.
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