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- W2013058368 abstract "Summary A new method of separation of uranyl ions from di-, tri- and tetravalent cations such as thorium, zirconium, cerium(IV) and/or lanthanides(III) involving phosphoric acid medium is described in this paper. The process is based on the difference of solubility between various phosphates: M 2 (PO 4 ) 2 (HPO 4 )·H 2 O, M(HPO 4 ) 2 ·H 2 O, M(OH)PO 4 (where M is a tetravalent cation) or APO 4 · n H 2 O (where A is a trivalent cation) on the one hand, and the uranyl phosphate pentahydrate (UO 2 ) 3 (PO 4 ) 2 ·5H 2 O, on the other hand. Taking into account the associated solubility constants, the conditions of separation were calculated then experimented for a mixture of Th 4+ , Ce 4+ (as a plutonium surrogate), Zr 4+ , La 3+ , Ba 2+ , Sr 2+ and UO 2 2+ . Tetravalent and trivalent cations phosphates were precipitated in 2 mol L −1 nitric acid medium while uranyl ion and divalent cations remained in the solution. In a second step, (UO 2 ) 3 (PO 4 ) 2 ·5H 2 O was precipitated at pH ≈ 1.5 and thereby separated from divalent cations present in the solution." @default.
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- W2013058368 date "2006-08-01" @default.
- W2013058368 modified "2023-10-17" @default.
- W2013058368 title "Separation of uranium(VI) from tri- and tetravalent elements in phosphoric acid solutions" @default.
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- W2013058368 doi "https://doi.org/10.1524/ract.2006.94.8.461" @default.
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