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- W2013092331 abstract "The development of a general organocatalyst for the α-functionalization of aldehydes, via an enamine intermediate, is presented. Based on optically active α,α-diarylprolinol silyl ethers, the scope and applications of this catalyst for the stereogenic formation of C−C, C−N, C−F, C−Br, and C−S bonds are outlined. The reactions all proceed in good to high yields and with excellent enantioselectivities. Furthermore, we will present mechanistic insight into the reaction course applying nonlinear effect studies, kinetic resolution, and computational investigations leading to an understanding of the properties of the α,α-diarylprolinol silyl ether catalysts." @default.
- W2013092331 created "2016-06-24" @default.
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- W2013092331 date "2005-12-01" @default.
- W2013092331 modified "2023-10-11" @default.
- W2013092331 title "A General Organocatalyst for Direct α-Functionalization of Aldehydes: Stereoselective C−C, C−N, C−F, C−Br, and C−S Bond-Forming Reactions. Scope and Mechanistic Insights" @default.
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- W2013092331 doi "https://doi.org/10.1021/ja056120u" @default.
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