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- W2013111017 abstract "Two-dimensional systems such as surfaces and molecular monolayers exhibit a multitude of intriguing phases and complex transitions. Ultrafast structural probing of such systems offers direct time-domain information on internal interactions and couplings to a substrate or bulk support. We have developed ultrafast low-energy electron diffraction and investigate in transmission the structural relaxation in a polymer/graphene bilayer system excited out of equilibrium. The laser-pump/electron-probe scheme resolves the ultrafast melting of a polymer superstructure consisting of folded-chain crystals registered to a free-standing graphene substrate. We extract the time scales of energy transfer across the bilayer interface, the loss of superstructure order, and the appearance of an amorphous phase with short-range correlations. The high surface sensitivity makes this experimental approach suitable for numerous problems in ultrafast surface science." @default.
- W2013111017 created "2016-06-24" @default.
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- W2013111017 date "2014-07-11" @default.
- W2013111017 modified "2023-10-17" @default.
- W2013111017 title "Ultrafast low-energy electron diffraction in transmission resolves polymer/graphene superstructure dynamics" @default.
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- W2013111017 doi "https://doi.org/10.1126/science.1250658" @default.
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