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• W2013169996 abstract "Using dynamical density functional theory we calculate the speed of solidification fronts advancing into a quenched two-dimensional model fluid of soft-core particles. We find that solidification fronts can advance via two different mechanisms, depending on the depth of the quench. For shallow quenches, the front propagation is via a nonlinear mechanism. For deep quenches, front propagation is governed by a linear mechanism and in this regime we are able to determine the front speed via a marginal stability analysis. We find that the density modulations generated behind the advancing front have a characteristic scale that differs from the wavelength of the density modulation in thermodynamic equilibrium, i.e., the spacing between the crystal planes in an equilibrium crystal. This leads to the subsequent development of disorder in the solids that are formed. For the one-component fluid, the particles are able to rearrange to form a well-ordered crystal, with few defects. However, solidification fronts in a binary mixture exhibiting crystalline phases with square and hexagonal ordering generate solids that are unable to rearrange after the passage of the solidification front and a significant amount of disorder remains in the system." @default.
• W2013169996 created "2016-06-24" @default.
• W2013169996 creator A5065432194 @default.
• W2013169996 creator A5065649147 @default.
• W2013169996 creator A5068202262 @default.
• W2013169996 creator A5072485128 @default.
• W2013169996 date "2014-10-17" @default.
• W2013169996 modified "2023-10-15" @default.
• W2013169996 title "Solidification in soft-core fluids: Disordered solids from fast solidification fronts" @default.
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• W2013169996 doi "https://doi.org/10.1103/physreve.90.042404" @default.
• W2013169996 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25375507" @default.

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