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• W2013190267 startingPage "953" @default.
• W2013190267 abstract "Lattice vibrations in orthorhombic Ta${mathrm{S}}_{3}$ have been investigated by polarized Raman scattering above and below the charge-density-wave (CDW) phase-transition temperature of 218 K. Below ${T}_{c}$, satellite peaks become clear on the lower-energy slopes of the dominant peaks and increase the intensity with decreasing temperature. The main peaks at room temperature decrease the intensity and shift to the higher-energy side below ${T}_{c}$. This one-dimensional material consists of 24 trigonal prismatic chains in the unit cell. Each chain which has different tendency for the CDW formation is assumed to give one of the satellite peaks. In the chains with large CDW amplitude, the decrease in the number of free carriers due to the formation of the CDW gap at the Fermi level leads to a decrease in the scattering intensity from the intraband process as well as an increase in the phonon energy. The temperature dependence of the scattering intensity is compared with the calculated intraband scattering intensity, which is proportional to the bare electronic susceptibility of the electron gas in the conduction band with the CDW gap." @default.
• W2013190267 created "2016-06-24" @default.
• W2013190267 creator A5055575436 @default.
• W2013190267 date "1984-01-15" @default.
• W2013190267 modified "2023-09-28" @default.
• W2013190267 title "Effect of the charge-density-wave gap on the Raman spectra in orthorhombic Ta<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>S</mml:mi></mml:mrow><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>" @default.
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• W2013190267 doi "https://doi.org/10.1103/physrevb.29.953" @default.
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