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- W2013217800 abstract "The spectroscopy of SF6, excited in its quasi-continuum by IR multiphoton absorption, has been recorded by IR fluorescence from ν = 700 to 1300 cm−1 with a highly sensitive device. The far resonance fluorescence exhibits structures directly connected to the intramolecular couplings. A model of couplings has been developed, the parameters of which are fixed by the experimental results. The strongest couplings (orders k = 3 and 4) have a density so low that they produce only a perturbative redistribution of the ν3 mode. The dissipative redistribution is produced by the highest orders k⩾5 and can be represented by a half-linewidth γd∼1.5 cm−1 for Evib∼ 15,000 cm−1. The onset of the SF6 quasi-continuum is also predicted by the model, with characteristics in full agreement with published data." @default.
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- W2013217800 date "1994-05-01" @default.
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- W2013217800 title "Fluorescence from SF6 in highly excited vibrational states: An overview" @default.
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- W2013217800 doi "https://doi.org/10.1016/0584-8539(94)80146-0" @default.
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