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• W2013268835 abstract "Molecular dynamics (MD) simulations of cis-1,4-polybutadiene in bulk amorphous state were performed to elucidate the origin of a fast relaxation process observed by quasielastic neutron scattering (QENS) measurements. The details of the torsional motion for each dihedral angle were investigated with the torsional auto- and cross-correlation functions for several temperatures in this study. Temperature dependence of the correlation between the torsional autocorrelation and cross-correlation functions is also evaluated. The origin of the fast process of cis-1,4-polybutadiene is found to be mainly the cooperative conformational transitions of two dihedral angles located at both sides of the CH2–CH2 bond when the bond is in the trans conformation. The cooperative conformational transitions exhibit even below the glass transition temperature of cis-1,4-polybutadiene. The cooperative motion appears at about 50 K below the glass transition temperature, corresponding to the Vogel–Fulcher temperature." @default.
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• W2013268835 date "2002-02-01" @default.
• W2013268835 modified "2023-09-27" @default.
• W2013268835 title "Molecular dynamics simulation of cis-1,4-polybutadiene. 2. Chain motion and origin of the fast process" @default.
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• W2013268835 doi "https://doi.org/10.1016/s0032-3861(01)00629-2" @default.
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