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• W2013371390 abstract "Tetratomic tetrahedral main-group clusters have four or six (but not five) skeletal pairs, an exception to the (n + 1) rule for closo clusters. A general group-theoretical criterion, based on the pairing principle in Stone's tensor surface harmonic (TSH) theory, is presented for symmetry-induced departures from the (n + 1) rule. A count of (n + 2) or n skeletal pairs is forced by symmetry for: (i) T- or Td-clusters with an odd number of sets of four equivalent cage atoms, and (ii) Cm or Cmv (m ⩾ 3) clusters with an odd number of cage atoms on the Cm-axis. Three such cases, BnHn or BnHn4−, are found among the hypothetical supraicosahedral closo boranes proposed by Brown and Lipscomb (n = 16,19 or 22). Extended Hückel calculations show that the TSH pattern applies to the whole series of closo boranes (n ̌ 24). Charges of + 4, −8 and −2 are discussed for a very large B32H32 q cluster." @default.
• W2013371390 created "2016-06-24" @default.
• W2013371390 creator A5025309888 @default.
• W2013371390 date "1985-01-01" @default.
• W2013371390 modified "2023-10-14" @default.
• W2013371390 title "The pairing principle in tensor surface harmonic theory: Electron counts of large closo boranes" @default.
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• W2013371390 doi "https://doi.org/10.1016/s0277-5387(00)86734-0" @default.
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