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• W2013383405 abstract "We present a comparison between accurate ab initio calculations and a high-quality experimental data set (1986--2002) of electric-field gradients of $mathrm{Cd}$ at different sites on $mathrm{Ni}$, $mathrm{Cu}$, $mathrm{Pd}$, and $mathrm{Ag}$ surfaces. Experiments found a systematic rule to assign surface sites on (100) and (111) surfaces based on the main component of the electric-field gradient, a rule that does not work for (110) surfaces. Our calculations show that this particular rule is a manifestation of a more general underlying systematic behavior. When looked upon from this point of view, (100), (111) and (110) surfaces behave in precisely the same way. The physical mechanism behind the systematics of the EFG for other $5sp$ impurities $(mathrm{Cd}text{ensuremath{-}}mathrm{Ba})$ at different fcc surfaces sites is revealed, showing in a natural way why the first half of the $5mathit{p}$ elements shows a coordination dependence that is opposite with respect to the second half." @default.
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• W2013383405 date "2004-10-29" @default.
• W2013383405 modified "2023-09-26" @default.
• W2013383405 title "Coordination dependence of hyperfine interactions at impurities on fcc metal surfaces. I. Electric-field gradient" @default.
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• W2013383405 doi "https://doi.org/10.1103/physrevb.70.155418" @default.
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