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- W2013410784 abstract "Methyl-radical and atomic hydrogen adsorption on C(111) have been studied by infrared-visible sum-frequency vibrational spectroscopy. Methyl iodide, di-tert-butyl-peroxide, and methane passing through a hot filament are used to produce methyl radicals (${mathrm{CH}}_{3}$). Low-energy ${mathrm{CH}}_{3}$ from pyrolytic dissociation at ensuremath{sim}800 ifmmode^circelsetextdegreefi{}C adsorb intact on the surface, but with surface annealing above 350 ifmmode^circelsetextdegreefi{}C, convert to tetrahedrally bonded CH. High-energy ${mathrm{CH}}_{3}$ produced at ensuremath{sim}1800 ifmmode^circelsetextdegreefi{}C convert readily to CH upon adsorption. Co-dosing a high-temperature (ensuremath{sim}800 ifmmode^circelsetextdegreefi{}C) C(111) substrate with hydrogen and methane via a hot filament at ensuremath{sim}1800 ifmmode^circelsetextdegreefi{}C yields only the stable tetrahedrally-bonded CH-species on the surface. They appear to stabilize the diamond surface structure. The coverage is not full, leaving sites open for ${mathrm{CH}}_{3}$ to adsorb and convert to CH as is necessary for chemical vapor deposition diamond growth. textcopyright{} 1996 The American Physical Society." @default.
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- W2013410784 date "1996-09-15" @default.
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- W2013410784 title "Interactions of hydrogen and methyl radicals with diamond C(111) studied by sum-frequency vibrational spectroscopy" @default.
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- W2013410784 doi "https://doi.org/10.1103/physrevb.54.8243" @default.
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