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- W2013458184 abstract "The interaction of formic acid with amorphous manganese oxide (AMO) is investigated using in situ photoelectron and infrared spectroscopy techniques. Soft X-ray photoelectron spectroscopy (sXPS) and in situ FTIR illustrate two possible modes of formate bound species at the AMO surface. Two peaks in the IR region from 1340−1390 cm−1 are indicative of formate species bound to the surface in a bidentate configuration. However, a 224 cm−1 band gap between νsOCO and νasOCO suggests formate is bound in a bridging configuration. Temperature-programmed desorption studies confirm the formate bound species desorbs as carbon dioxide from the surface at multiple binding sites. At temperatures above 700 K, the presence of K+···OC complex suggests the bound species interacts at vacant sites related to framework oxygen and cation mobility." @default.
- W2013458184 created "2016-06-24" @default.
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- W2013458184 date "2010-11-05" @default.
- W2013458184 modified "2023-09-27" @default.
- W2013458184 title "Reaction of Formic Acid over Amorphous Manganese Oxide Catalytic Systems: An In Situ Study" @default.
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- W2013458184 doi "https://doi.org/10.1021/jp104629j" @default.
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