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- W2013488082 abstract "The application of a Pb2+ conducting solid electrolyte (Pb-β‘ ‘ alumina) to electrochemical control of catalyst performance is reported. XPS data show that pumping of Pb to/from a thin film platinum catalyst from/to the solid electrolyte provides a controlled, reversible, and reproducible way of altering the surface composition of the resulting Pt/Pb surface alloy under conditions of acetylene hydrogenation. With increasing Pb concentration a large increase in partial hydrogenation selectivity occurs from 20% (pure Pt surface) to 85% (∼26% Pb surface alloy). The results demonstrate that the surface composition and catalytic performance of bimetallic alloy catalysts can be dramatically and reversibly altered under working conditions by electrochemical means." @default.
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- W2013488082 date "2002-09-07" @default.
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- W2013488082 title "In Situ Control of the Composition and Performance of a Bimetallic Alloy Catalyst: The Selective Hydrogenation of Acetylene over Pt/Pb" @default.
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- W2013488082 doi "https://doi.org/10.1021/jp021296t" @default.
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