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• W2013608837 abstract "Photodissociation of pyrimidine at 193 and 248nm was investigated separately using vacuum ultraviolet photoionization at 118.4 and 88.6nm and multimass ion imaging techniques. Six dissociation channels were observed at 193nm, including C4N2H4→C4N2H3+H and five ring opening dissociation channels, C4N2H4→C3NH3+HCN, C4N2H4→2C2NH2, C4N2H4→CH3N+C3NH, C4N2H4→C4NH2+NH2, and C4N2H4→CH2N+C3NH2. Only the first four channels were observed at 248nm. Photofragment translational energy distributions and dissociation rates indicate that dissociation occurs in the ground electronic state after internal conversion at both wavelengths. The dissociation rates were found to be &gt;5×107 and 1×106s−1 at 193 and 248nm, respectively. Comparison with the potential energies from ab initio calculations have been made." @default.
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• W2013608837 date "2006-02-22" @default.
• W2013608837 modified "2023-10-07" @default.
• W2013608837 title "Photodissociation dynamics of pyrimidine" @default.
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• W2013608837 doi "https://doi.org/10.1063/1.2174011" @default.
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