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- W2013726022 abstract "In this paper we present a kinetic analysis of the consecutive photoreaction scheme A⇄hνB→hνC assuming the reaction is carried out in a continuous flow stirred tank reactor (CSTR). The reactor is kept at constant temperature and fed with reactant A at a constant flow rate. A numerical analysis of the model’s stationary states reveals a range of constraints for which the system possesses multiple steady states. The observed bistability depends strongly on the rate constant of the B→A reaction k2 . It is typically observed when k2 is much larger than the other rate constants. Our numerical calculations also reveal a marked dependency on parameters such as the molar absorptivities and the irradiation intensity I0 . Interestingly, multiple steady states are only observed for intermediate values of I0 . Analytical approximations are obtained for the stationary states in the limit where the end-product C does not absorb light. These approximations are used to clarify the mechanism responsible for the light-induced instability." @default.
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- W2013726022 title "Bistability in isothermal photochemical systems: The A⇄<sup><i>h</i>ν</sup>B→<sup><i>h</i>ν</sup>C reaction in a continuous flow stirred tank reactor" @default.
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- W2013726022 doi "https://doi.org/10.1063/1.455143" @default.
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