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- W2013775871 abstract "We report the combined measurements of the dc susceptibility ${ensuremath{chi}}_{0}$, the ac susceptibility ${ensuremath{chi}}^{ensuremath{'}}$, and the NMR relaxation rate ${T}_{1}^{ensuremath{-}1}$ for the molecular-based heterometallic single-chain magnet ${[mathrm{Mn}(text{saltmen})]}_{2}[mathrm{Ni}{(mathrm{pao})}_{2}{(mathrm{py})}_{2}]{(mathrm{P}{mathrm{F}}_{6})}_{2}$. At low temperatures, this system is well described by a one-dimensional array of effective spin $S=3$ chains comprising the ${mathrm{Mn}}^{III}text{ensuremath{-}}{mathrm{Ni}}^{II}text{ensuremath{-}}{mathrm{Mn}}^{III}$ trimers and treated as the $S=3$ Ising chain with the single-ion term (Blume-Capel model). Using the exact solution of the model and based on the picture that the random motion of the local domain walls dominates the low-temperature spin dynamics, we succeeded in reproducing the experimental results of the dc susceptibility ${ensuremath{chi}}_{0}$, the ac susceptibility ${ensuremath{chi}}^{ensuremath{'}}$, and the $^{19}mathrm{F}text{ensuremath{-}}mathrm{NMR}$ relaxation rate ${T}_{1}^{ensuremath{-}1}$ in a consistent manner." @default.
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- W2013775871 date "2006-12-15" @default.
- W2013775871 modified "2023-10-15" @default.
- W2013775871 title "Spin correlation and relaxational dynamics in molecular-based single-chain magnets" @default.
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- W2013775871 doi "https://doi.org/10.1103/physrevb.74.224419" @default.
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