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• W2013806773 abstract "Experimental results describing the product distribution during the reduction of NO by H2 on Pt/Al2O3 and Pt/BaO/Al2O3 catalysts are presented in the temperature range 30–500 °C and H2/NO feed ratio range of 0.9–2.5. A microkinetic model that describes the kinetics of NO reduction by H2 on Pt/Al2O3 is proposed and most of the kinetic parameters are estimated from either literature data or from thermodynamic constraints. The microkinetic model is combined with the short monolith flow model to simulate the conversions and selectivities corresponding to the experimental conditions. The predicted trends are in excellent qualitative and reasonable quantitative agreement with the experimental results. Both the model and the experiments show that N2O formation is favored at low temperatures and low H2/NO feed ratios, N2 selectivity increases monotonically with temperature for H2/NO feed ratios of 1.2 or less but goes through a maximum at intermediate temperatures (around 100 °C) for H2/NO feed ratios 1.5 or higher. Ammonia formation is favored for H2/NO feed ratios of 1.5 or higher and intermediate temperatures (100–350 °C) buts starts to decompose at a temperature of 400 °C or higher. The microkinetic model is used to determine the surface coverages and explain the trends in the experimentally observed selectivities." @default.
• W2013806773 created "2016-06-24" @default.
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• W2013806773 date "2008-01-01" @default.
• W2013806773 modified "2023-09-26" @default.
• W2013806773 title "Experimental and microkinetic modeling of steady-state NO reduction by H2 on Pt/BaO/Al2O3 monolith catalysts" @default.
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• W2013806773 doi "https://doi.org/10.1016/j.apcatb.2007.08.008" @default.
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