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- W2013848473 abstract "Both electron tunneling spectroscopy (IETS) and phonon subpeaks in resonant tunneling probe electronic-vibrational coupling in electron transport through single molecules. Higher phonon harmonics are often seen in resonant tunneling but not in IETS. For the case of subresonant (a.k.a. inelastic or virtual) electron transport, higher harmonics are shown to be damped by unexpected small factors beyond the powers of electron-vibration coupling constant λ. We calculate explicitly for a standard model the strength of higher harmonics in transport to understand these additional small factors, which result from an orthogonality constraint. Two mechanisms greatly increase the size of secondary peaks in subresonant transport: coupling between electron transport and spatial motion of the molecule, and the pumping of higher vibrational modes of the molecule when vibrational excitations do not completely relax between electron transits." @default.
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- W2013848473 date "2004-06-01" @default.
- W2013848473 modified "2023-09-27" @default.
- W2013848473 title "HIGHER HARMONICS OF ELECTRONIC-VIBRATIONAL COUPLING IN SUBRESONANT AND RESONANT TRANSPORT IN SINGLE-MOLECULE DEVICES" @default.
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- W2013848473 doi "https://doi.org/10.1142/s0219581x0400205x" @default.
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