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- W2013903513 abstract "The ligand exchange reaction between free and coordinated carbonate on 242PuVIO2(13CO3)34− and 243AmVIO2(13CO3)34− systems was examined by variable temperature 13C pulsed nuclear magnetic resonance (NMR) techniques. A modified Carr-Purcell-Meiboom-Gill NMR pulse sequence was used for the experimental determination of ligand exchange parameters for paramagnetic actinide complexes. Eyring analysis provided activation parameters of ΔG295‡ = 53 kJ M−1, ΔH‡ = 35 kJ M−1and ΔS295‡ = −61 J M−1K−1 for the plutonyl triscarbonate system, suggesting an associative transition state for the plutonyl(VI) carbonate self-exchange reaction." @default.
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- W2013903513 date "1993-03-01" @default.
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- W2013903513 title "13C NMR characterization of actinyl(VI) carbonate complexes in aqueous solution" @default.
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- W2013903513 doi "https://doi.org/10.1016/0925-8388(93)90319-i" @default.
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