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- W2014177227 abstract "The dissociation rate of CO2 has been measured for temperatures of 3500° to 6000°K. The rate of disappearance of CO2 behind shock waves in CO2–N2 and CO2–Ar gas mixtures was monitored by observing the infrared radiation from the CO2 4.3-μ fundamental vibration band. The dissociation rates expressed in the classical collision theory for 1% CO2 in both Ar and N2 are kAr = (9.71) (10—14) (D/kT)4.38 exp (—D/kT) and kN2 = (3.27) (10—14) (D/kT)4.72 exp (—D/kT) where D = 5.5 eV is the CO2 dissociation energy, k is the Boltzmann constant, and T is the absolute temperature. The same data fit to an Arrhenius equation yields the rate constants kAr = (4.79) (10—13) T½ exp (—3.24 eV/kT) and kN2 = (4.07) (10—13) T½ exp (—3.23 eV/kT). The dissociation rate is not altered within the experimental error by (a) increasing the CO2 concentration up to 10%, (b) adding either CO of H2O to the gas for concentrations of these gases up to 2%, (c) making the dissociation measurement at different wavelengths or pass bands within the 4.3-μ band, or (d) making the dissociation measurement by observing the radiation from the CO2 2.7-μ combination bands." @default.
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- W2014177227 date "1964-09-15" @default.
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- W2014177227 title "Carbon Dioxide Dissociation at 3500° to 6000°K" @default.
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- W2014177227 doi "https://doi.org/10.1063/1.1726165" @default.
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