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- W2014230731 abstract "A chain model in a cubic lattice has been used to examine the effect of flexibility and the mechanism of the latter on local density and the micro-structure of macromolecules in solutions. The average number of intramolecular collisions, the distribution of loops, the average length of the rigid and of colliding parts, the distribution by length in “good” and “poor” solvents, have been calculated. The mode by which intramolecular collisions are realized in the various mechanisms of chain flexing has been analysed. The local density and the steric micro-structure of flexible chains are determined by the behaviour of short chain parts several bonds long. Where it is difficult for the chains to fold up, a small local density is typical, also a cross-shaped position of the interacting parts, and a slight dependence of the geometrical and thermodynamic characteristics on solvent quality. The existence of mobile reinforcements inside the chains results in an appearance of folding structure centres in solvents near the θ point, of large local densities in flexible chains, of an θ-temperature depending on rigidity, and of a larger dependence of internal characteristics of the chain on solvent quality. Intramolecular pseudo-crystals will also appear in the fairly rigid macromolecules in “poor” solvents near the θ-point." @default.
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- W2014230731 date "1976-01-01" @default.
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- W2014230731 title "The local density and the micro-structure of polymers investigated by the Monte Carlo method" @default.
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- W2014230731 doi "https://doi.org/10.1016/0032-3950(76)90099-x" @default.
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