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- W2014232577 abstract "The aims of this paper are to propose, construct and analyse microscopic kinetic models for the emergence of long chains of RNA from monomeric �-D-ribonucleotide precursors in prebiotic circumstances. Our theory starts out from similar but more general chemical assumptions to those of Eigen [1], namely that catalytic replication can lead to a large population of long chains. In particular, our models incorporate the possibility of (i) direct chain growth, (ii) template-assisted synthesis and (iii) catalysis by RNA replicase ribozymes, all with varying degrees of efficiency. However, in our models the reaction mechanisms are kept ‘open’; we do not assume the existence of closed hypercycles which sustain a population of long chains. Rather it is the feasibility of the initial emergence of a self-sustaining set of RNA chains from monomeric nucleotides which is our prime concern. Moreover, we confront directly the central nonlinear features of the problem, which have often been overlooked in previous studies. Our detailed microscopic kinetic models" @default.
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- W2014232577 date "1999-05-01" @default.
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- W2014232577 title "The Origin of the RNA World: A Kinetic Model" @default.
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- W2014232577 doi "https://doi.org/10.1021/jp983159v" @default.
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