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• W2014298384 abstract "Compounds containing cations with a valence electron configuration that can formally be described as (n−1)d10ns0 (Cu+, Ag+, Au+, Hg2+) exhibit a variety of unusual structural properties, e.g. low coordination numbers and short cation-cation distances. The incorporation of d electrons from the closed d10 sub-shell has been debated for a long time as a reason for this extraordinary behaviour. Ag L3 XANES spectra of oxidic silver(I) compounds exhibit a prominent peak at the rising edge. By comparison with the XANES spectrum of a Ag(III) periodate complex this peak is assigned to a transition from initial 2p states to 4d final states, proving that in oxidic Ag(I) compounds the closed-shell configuration 4d10 is broken. The intensity of the peak signalling unoccupied 4d states is related to the degree of covalent bonding in a compound." @default.
• W2014298384 created "2016-06-24" @default.
• W2014298384 creator A5040021405 @default.
• W2014298384 date "1992-01-01" @default.
• W2014298384 modified "2023-09-28" @default.
• W2014298384 title "Bonding in silver-oxygen compounds from Ag L3 XANES spectroscopy" @default.
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• W2014298384 doi "https://doi.org/10.1016/0038-1098(92)90506-5" @default.
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