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- W2014352261 abstract "Abstract CH-stretching modes were first excited by picosecond infrared pulses and the generated excess population was monitored by anti-Stokes scattering of subsequent ultrashort probe pulses. Experimental data are reported on five molecules: CHCl 3 , CH 2 Cl 2 , CH 3 CCl 3 , CH 3 CH 2 OH, and CH 3 I in the neat liquid and/or in solutions of CCl 4 . The observed time constants vary between 1 and 100 ps depending upon the individual molecule and surrounding. Theoretical calculations show that rotational coupling, Fermi resonance, Coriolis coupling, and resonance energy transfer can strongly effect the vibrational population lifetime. The relevance of these processes is quite different for the various molecules investigated." @default.
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- W2014352261 date "1978-07-01" @default.
- W2014352261 modified "2023-10-12" @default.
- W2014352261 title "Vibrational population lifetimes of polyatomic molecules in liquids" @default.
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- W2014352261 doi "https://doi.org/10.1016/0301-0104(78)85126-x" @default.
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