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• W2014379842 abstract "Abstract The adsorption of NO onto Ni/SiO 2 catalyst has been investigated at 77 and 296 K at various pressures by EPR spectroscopy. The principal steps of NO disproportionation involve coordination of NO molecule with concomitant formation of paramagnetic mono {Ni II 3c –NO } 9 /SiO 2 and diamagnetic dinitrosyl species {Ni 2c –(NO) 2 } 10 /SiO 2 , reduction of nickel through inner-sphere ligand-to-metal electron transfer leading to {Ni I 3c –NO + } 9 /SiO 2 , formation of {Ni 3c –NO 2 } 9 /SiO 2 complex via metal-oxo intermediate, and spillover of the NO 2 ligand onto silica. The key reaction intermediates have been isolated and identified. Their assignment and molecular structure have been ascertained by DFT calculations." @default.
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• W2014379842 date "2006-05-01" @default.
• W2014379842 modified "2023-09-25" @default.
• W2014379842 title "EPR and DFT study of NO interaction with Ni/SiO2 catalyst: Insight into mechanistic steps of disproportionation process promoted by tripodal surface nickel complex" @default.
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• W2014379842 doi "https://doi.org/10.1016/j.cattod.2006.01.016" @default.
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