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• W2014430360 abstract "This paper describes a new concept of dense, dual-phase membrane consisting of two phases conducting, respectively, CO32- and electrons for selective permeation of CO2 and O2 at high temperatures. Membranes with a molten carbonate phase in a porous stainless-steel support were synthesized by a direct infiltration method. Membrane preparation conditions were optimized to obtain stable, gas-tight dual-phase membranes at high temperatures (>450 °C). The dual-phase membranes exhibit low single-gas permeance for pure CO2 and N2 (<5 × 10-9 mol s-1 m-2 Pa-1) in 450−650 °C but substantially higher CO2 permeance for CO2 mixed with O2 at high temperatures. CO2, after interacting with O2, transports through the molten carbonate phase in a form of CO32-, with electrons transporting through the porous metal support. With further improvement, the dual-phase membranes may offer application in producing O2-enriched CO2 streams for the oxyfuel combustion process. The concept can be also extended to prepare CO2 perm-selective dense membranes for high-temperature CO2 separation." @default.
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• W2014430360 date "2005-09-13" @default.
• W2014430360 modified "2023-10-03" @default.
• W2014430360 title "Dual-Phase Metal−Carbonate Membrane for High-Temperature Carbon Dioxide Separation" @default.
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• W2014430360 doi "https://doi.org/10.1021/ie0503141" @default.
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