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• W2014511551 abstract "VII[TCNE]-z[TCNE]2-1-z/2 (1 < z < 2) is the simplest formulation for the inhomogeneous and nonstoichiometric V[TCNE]x (x = 1 + z/2) room temperature magnet. This is based upon consideration of all of the surface, IR, elemental composition, and magnetic data. A limiting z = 1 2-D, layered structural motif with layers of μ4-[TCNE]− bonded to four VII sites bridged by diamagnetic μ4-[TCNE]2− is described, and is sufficient to account for the observed Tc exceeding room temperature and the observed relatively high conductivity. The z = 2 limiting structure with the same layers, but bridged by S = 1/2 μ-[TCNE]− is identified and provides for a 3-D magnetic structure. Nonetheless, the magnet does not diffract, and the featureless morphology observed from TEM studies suggests that it is a glassy material. Attempts to grow crystalline V[TCNE]x by several slow diffusion methods were unsuccessful, and did not result is a magnetically ordered material. This suggests that the V[TCNE]x room temperature magnet is a kinetic phase, and preparing a crystalline kinetic product will be challenging." @default.
• W2014511551 created "2016-06-24" @default.
• W2014511551 creator A5079379110 @default.
• W2014511551 date "2009-06-01" @default.
• W2014511551 modified "2023-10-16" @default.
• W2014511551 title "Oliver Kahn Lecture: Composition and structure of the V[TCNE]x (TCNE=tetracyanoethylene) room-temperature, organic-based magnet – A personal perspective" @default.
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• W2014511551 doi "https://doi.org/10.1016/j.poly.2008.11.030" @default.
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