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- W2014518342 abstract "A continuous supersonic molecular beam of small methanol clusters is crossed by the radiation of a pulsed CO2 laser. Subsequent scattering by a secondary He beam disperses the cluster beam and allows the off-axis detection of selected cluster species, undisturbed by ionizer fragmentation artifacts. In the region of the ν8 CO stretching vibration, the dependence of IR photon absorption on laser frequency and fluence is investigated as a function of cluster size. The predissociation spectrum of the dimer shows two distinct peaks at 1026.5 and 1051.6 cm−1 which correspond to the excitation of the two non-equivalent monomers in the dimer. The trimer spectrum features one single peak centered at 1042.2 cm−1. This is consistent with a cyclic structure in which all three methanol molecules are equivalent. Higher cluster spectra are characterized by single peaks gradually blue-shifted with respect to the trimer line." @default.
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- W2014518342 date "1988-03-01" @default.
- W2014518342 modified "2023-10-12" @default.
- W2014518342 title "Infrared photodissociation of small methanol clusters" @default.
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- W2014518342 doi "https://doi.org/10.1016/0009-2614(88)87135-5" @default.
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