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- W2014538692 abstract "Henderson [Phys. Rev. A 32, 2336 (1985)] has proposed that the critical exponent for adsorption should be either ensuremath{gamma} or ensuremath{gamma}/2, where ensuremath{gamma} is the (bulk) compressibility exponent. It is shown that both results are artifacts of the mean spherical approximation (MSA) employed by Henderson. The MSA, and closely related closures of the wall-particle Ornstein-Zernike equation, are essentially linear-response approximations which neglect nonlinearities that are crucial in critical adsorption, even at the mean-field level. Our argument is made explicit by re-deriving the correct (Fisher--de Gennes) exponent ensuremath{nu}-ensuremath{beta} and illustrating the failings of linearized treatments. Since the latter also fail to describe complete wetting, their validity is restricted to states well removed from bulk two-phase coexistence." @default.
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- W2014538692 date "1986-10-01" @default.
- W2014538692 modified "2023-10-16" @default.
- W2014538692 title "Comment on ‘‘Simple theory for the critical adsorption of a fluid’’" @default.
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- W2014538692 doi "https://doi.org/10.1103/physreva.34.3504" @default.
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