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- W2014652316 abstract "Metal-ligand interactions with various proteins form in vivo metal assemblies. In recent years, metallosupramolecular approaches have been utilized to forge an assortment of fascinating two- and three-dimensional nano-architectures and macroscopic materials, such as metal-ligand coordination polymeric materials, have promise in artificial systems. However to the best of our knowledge, the self-assembly of macroscopic materials through metal-ligand interactions has yet to be reported. Herein we demonstrate a gel assembly formed via metal-ligand interactions using polyacrylamide modified with Fe-porphyrin and L-histidine moieties. The stress values for the assembly increase as the concentration of Fe-porphyrin or L-histidine in the gels increases. Moreover, agitation of Fe-porphyrin gel, Zn-porphyrin gel and L-histidine gel in an 80 mM Tris-acetate buffer (pH 9.0) results in selective adhesion of the Fe-porphyrin gel to the L-histidine gel based on the affinities of Fe-porphyrin and Zn-porphyrin with L-histidine." @default.
- W2014652316 created "2016-06-24" @default.
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- W2014652316 date "2013-02-07" @default.
- W2014652316 modified "2023-09-26" @default.
- W2014652316 title "Reversible self-assembly of gels through metal-ligand interactions" @default.
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- W2014652316 doi "https://doi.org/10.1038/srep01243" @default.
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