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• W2014707615 startingPage "6992" @default.
• W2014707615 abstract "The unimolecular dissociation of energy rich lithium cluster ions shows that Li+n dissociate by sequential atom or dimer loss. The binding energies of Li+n (n=4–42) generated in an evaporative ensemble are determined from unimolecular decay, within a well defined time window, and energy constraint. They present a sawtooth behavior vs cluster size less pronounced that it should be from a simple metal model. Odd–even alternation is superimposed on the sawtooth behavior, with odd sized cluster ions being more stable. Cohesive energies per atom of Li+n are deduced from these dissociation energies up to n=40 and from extended photo-induced measurements up to n=95. Cohesive energies per atom of neutral clusters Lin are derived by combining these ionic cohesive energies with the literature ionization potentials. The linearity of the neutral cluster cohesive energy vs the cluster surface to volume ratio permits a volume and a surface energy to be deduced. These values are compared to the bulk values." @default.
• W2014707615 created "2016-06-24" @default.
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• W2014707615 date "1994-10-15" @default.
• W2014707615 modified "2023-10-04" @default.
• W2014707615 title "Dissociation pathways and binding energies of lithium clusters from evaporation experiments" @default.
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• W2014707615 doi "https://doi.org/10.1063/1.468326" @default.
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