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- W2014714501 abstract "In a magnetic field, the wave number of a pump laser light polarized along the field was fixed to the isolated ${mathrm{Cs}}_{2}D{}^{1}{ensuremath{Sigma}}_{u}^{+}(v=46,J=54)ensuremath{leftarrow}X{}^{1}{ensuremath{Sigma}}_{g}^{+}(v=0,J=55)$ line, and the excitation spectrum of the dissociated $mathrm{Cs}(6p{}^{2}{P}_{3/2})$ atoms was measured by scanning the wave number of a probe laser light polarized perpendicular to the field. The population of each sublevel $6p{}^{2}{P}_{{3/2,m}_{j}}$ of the dissociated atoms was determined from the line intensities in the ${m}_{j}$-resolved excitation spectrum. The unequal population between the $6p{}^{2}{P}_{3/2,+|{m}_{j}|}$ and $6p{}^{2}{P}_{3/2,ensuremath{-}|{m}_{j}|}$ levels (atomic orientation) was observed and it was enhanced as the magnetic-field strength was increased. The atomic orientation is shown to be induced by the interference between the indirect predissociation, which occurs by a combination of the spin-orbit coupling of the $D{}^{1}{ensuremath{Sigma}}_{u}^{+}$ state with the ${(2)}^{3}{ensuremath{Pi}}_{0u}$ state and the L-uncoupling and Zeeman interactions between the ${(2)}^{3}{ensuremath{Pi}}_{0u}$ and dissociative ${(2)}^{3}{ensuremath{Sigma}}_{u}^{+}$ states, and the dissociation following a direct excitation to the ${(2)}^{3}{ensuremath{Sigma}}_{u}^{+}$ state, which is allowed by spin-orbit coupling of the ${(2)}^{3}{ensuremath{Sigma}}_{u}^{+}$ state with the $B{}^{1}{ensuremath{Pi}}_{u}$ state. It is demonstrated that the atomic orientation is produced by the photodissociation in the presence of an external magnetic field even when all degenerated molecular $M=J,dots{},0,dots{},ensuremath{-}J$ sublevels are excited by a light polarized linearly along the field." @default.
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- W2014714501 date "2003-06-27" @default.
- W2014714501 modified "2023-10-18" @default.
- W2014714501 title "Orientation observed by Zeeman spectra of dissociated atoms and the interference in photoexcitations" @default.
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- W2014714501 doi "https://doi.org/10.1103/physreva.67.062717" @default.
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