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- W2014748412 abstract "This paper reports the experimental examination of a novel device for the continuous, high-rate formation of a structure-H hydrate. The device is designed such that two precooled liquids, water and a hydrophobic large-molecule guest substance (LMGS), such as methylcyclohexane, are injected in the form of co-planar cylindrical jets into a hydrate-forming gas phase confined in a high-pressure chamber, where LMGS provides guest molecules to fit into the 51268 cages of a structure-H hydrate. The liquid jets collide, thereby forming a radially expanding sheet, which, in turn, sprinkles from its rim tiny water/LMGS compound droplets into the gas phase. Using methane and methylcyclohexane as the hydrate-forming gas and the LMGS, respectively, we have performed a series of hydrate-forming experiments to examine the operational function of the twin-jet device. The observed hydrate-formation behavior, including the rate of hydrate formation depending upon the degree of the LMGS cooling, is presented and discussed." @default.
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- W2014748412 date "2009-02-12" @default.
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- W2014748412 title "Forming a Structure-H Hydrate Using Water and Methylcyclohexane Jets Impinging on Each Other in a Methane Atmosphere" @default.
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- W2014748412 doi "https://doi.org/10.1021/ef800880f" @default.
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