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- W2014767106 abstract "A consistent method has been developed to calculate induced electromagnetic fields and optical transitions of electrons in a solid, in response to an incident laser beam of (circular) frequency $ensuremath{omega}$. The analysis is based upon the independent-particle Schrodinger equation for electrons and Maxwell's equations for the electromagnetic fields. General expressions for linear and bilinear currents as well as second-order optical transition probabilities have been derived. It is shown that the second-order transition probability, which is proportional to the fourth power in the incident field, contains two different types of terms, describing double-photon transitions of the incident frequency $ensuremath{omega}$ and single-photon transitions of the harmonic frequency $2ensuremath{omega}$. An estimate has been made to show that in the case of centrosymmetric solids like metals, the relative contribution due to the single second-harmonic photon transition is of the order ${(frac{{e}^{2}}{ensuremath{hbar}c})}^{2}ensuremath{ll}1$ in the optical region, compared with the double-fundamental-photon transition. However, in the case of solids lacking inversion symmetry, the contributions due to these two processes are estimated to be of the same order in magnitude." @default.
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- W2014767106 date "1966-05-13" @default.
- W2014767106 modified "2023-10-16" @default.
- W2014767106 title "Second-Order Optical Processes and Harmonic Fields in Solids" @default.
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- W2014767106 doi "https://doi.org/10.1103/physrev.145.500" @default.
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