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- W2014776867 abstract "The structure and catalytic property of molybdenum sulfide clusters encaged in NaY zeolite were investigated as a function of the composition of the host zeolite. The local structure of molybdenum sulfides was studied by means of MoK-edge XAFS. The local structure of intrazeolite molybdenum sulfide clusters depended on the Si/Al ratio of the host zeolite. Molybdenum sulfide dimer species were formed in NaY zeolites with a composition of 3.5 > Si/Al > 2.1. It is proposed that the structure of dimer clusters is reversibly transformed into a tetramer structure by an H2-treatment at 673 K. The intrinsic activity of molybdenum sulfide clusters for the HDS of thiophene decreased as the Mo–Mo distance of Mo2S4 dimer clusters increased." @default.
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- W2014776867 date "2007-04-01" @default.
- W2014776867 modified "2023-09-24" @default.
- W2014776867 title "Structure of molybdenum sulfide clusters encaged in zeolites: Effect of zeolite composition" @default.
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- W2014776867 doi "https://doi.org/10.1016/j.micromeso.2006.10.040" @default.
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