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• W2014796804 abstract "The loss of vibrational energy from gas phase T1 pyrazine molecules has been measured for thermal collisions with helium, argon, H2, SF6, and ground state pyrazine. Triplet pyrazine was prepared with a well defined vibrational energy of 5433 cm−1 through S1→T1 intersystem crossing following optical excitation to the 8a1 level of S1. The time‐dependent vibrational energy content of the excited pyrazine molecules was then deduced using a recently developed ‘‘direct’’ method involving the kinetics of subsequent T1→S0 intersystem crossing. For each of the collision partners studied, it was possible to find the average energy lost per gas kinetic collision for donor energies ranging from ca. 2000 to 5433 cm−1. The magnitudes of these energy losses generally increased with the mass and vibrational complexity of the relaxing collision partner. For vibrational energy contents near 5000 cm−1, relaxation of the triplet pyrazine was enhanced by factors of as much as 24 relative to S0 benzene at a similar vibrational..." @default.
• W2014796804 created "2016-06-24" @default.
• W2014796804 creator A5031525742 @default.
• W2014796804 creator A5045716690 @default.
• W2014796804 date "1993-04-15" @default.
• W2014796804 modified "2023-09-26" @default.
• W2014796804 title "Collisional vibrational relaxation of a triplet state: Energy‐dependent energy loss from <i>T</i>₁ pyrazine" @default.
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• W2014796804 doi "https://doi.org/10.1063/1.464825" @default.
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